My Zoho mail contacts are empty. I need my CRM contacts in there.

My Zoho mail contacts are empty. I need my CRM contacts in there.

How do I go about linking the the mail add-on with my CRM contacts?  I cannot export the full .csv file from Zoho CRM as there are more than 3000 contacts, and I cannot import anything larger than 1 Mb into my Zoho mail contacts.  What do I do?