Unable to send message;Reason:554 5.1.8 Email Outgoing Blocked.

I am getting the following error when sending email to anyone. Can this be fixed?

Unable to send message;Reason:554 5.1.8 Email Outgoing Blocked.

I do not send out bulk emails, like the error says, and so I don't understand why I am getting this.

My account is: brian.otto@zoho.com

I tried the Unblock Me link in the documentation and it didn't do anything, and just says this:

Your account brian.otto@zoho.com has been blocked due to security reasons.