Urgently!!!: Service Unavailable

Urgently!!!: Service Unavailable

Hello! After i got an email that said that my limit was full! i went to my email john@epsilonk.gr and i free up space... i can receive and sent emails from mail.zoho.com but in outlook i got all the time --ERR Service Unavailable..
can you please fix it or tell me how to fix it?

Thanks